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51.
为了定量计算陵区近海核电站排水管线泄漏情景下核素通过地下水途径向海洋环境的释放通量,以某近海核电站为例进行研究。首先,应用GOCAD软件建立三维地形地质模型,刻画地层的分布、剥蚀以及倾向等特点;然后,运用地下水数值模拟软件FEFLOW精细刻画丘陵区地下水系统的补给、径流和排泄特征;最后,以不被吸附滞留的核素3H和被吸附滞留的核素90Sr、137Cs为对象,通过实验测定了90Sr、137Cs在不同岩土介质中的分配系数,模拟计算了排水管线连续渗漏60 a后3H、90Sr、137Cs在地下水中的放射性分布及释放。结果表明:3H迁移速度基本与地下水流速一致,地下水中的最大放射性浓度为0.285 0 Bq/L,第20 000天时向收纳水域的释放通量达到最大值,约526 Bq/d;90Sr吸附性能相对较弱,最大迁移距离约80 m,地下水中的最大放射性浓度为0.032 1 Bq/L;137Cs吸附能力较强,相当长的时间内被滞留在管线附近,地下水中最大放射性浓度分别为6.840×10-3 Bq/L,释放通量为0 Bq/d。由弥散度的不确定分析可知,弥散度越大,地下水中3H的最大放射性浓度越小,向海洋环境的释放通量越多。 相似文献
52.
地下水中高浓度的铵态氮对生活饮用水安全及生态环境存在潜在威胁。相比较硝态氮,高浓度的铵态氮不仅有各种人为来源,天然沉积环境更是造成高铵地下水的主要成因。本文以城镇化快速发展的珠江三角洲为研究区,运用数理统计、主成分分析等方法深入探讨了研究区高铵地下水的赋存环境特征及驱动因素。结果表明,研究区地下水中NH4+质量浓度介于未检出~180 mg/L。研究区1539组地下水样品中,NH4+质量浓度大于10 mg/L的高铵地下水69组,其中含NH4+质量浓度大于30 mg/L的高铵"肥水"23组。对比2005-2008年历史水化学数据,2009-2018年新增建设用地孔隙含水层高铵地下水样品比例增加25%。高铵地下水呈斑块状分布于三角洲平原区第四系底部低洼的基底、洼地等退积层序发育的淤泥质含水层中。淤泥层等富含有机质和总有机碳的沉积层是珠江三角洲地区的"生铵层",有机氮的矿化是三角洲平原区城市化孔隙含水层中高铵地下水的主要驱动力。城镇化扩张引起生活污水及富铵工业废水的泄漏入渗是城乡结合部高铵地下水铵氮的重要来源。三角洲平原区中性至弱碱性富含有机质的还原环境是高铵地下水的主要成因。风化溶滤、阳离子交换吸附、海陆交互作用是珠江三角洲高铵地下水质演变的主要水文地球化学过程。 相似文献
53.
四川盆地三叠系地下水可划分出碎屑岩孔隙裂隙和碳酸盐岩岩溶裂隙两大储集类型。按此处构造开启程度和埋深条件等的不同,下中三叠统地下水有沉积变质水和渗入淋滤水两种基本成因类型,水动力特征各异。沉积变质水处于深埋封闭条件,受地静压力驱动控制;渗入淋滤水分布于背斜露头区和浅部地区,受静水压力驱动控制。并由此控制了盆地三叠系盐类的保存条件。 相似文献
54.
Yoko Fujikawa Daisuke Yoneda Atushi Minami Hiroshi Yashima Toshio Tonokai Sotoji Tani Masami Fukui Tatuhide Hamasaki Masataka Sugahara 《中国地球化学学报》2006,25(B08):113-113
Biological iron and manganese removal utilizing indigenous iron and manganese oxidizing bacteria (IRB hereafter) in groundwater can also be applied to arsenic removal according to our pilot-scale test. The arsenic removal probably occurred through sorption and complexation of arsenic to iron and manganese oxides formed by enzymic action of IRB. We investigated the chemical properties of iron and manganese oxides in IRB floc and the valence state of arsenic sorbed to the floc to clarify the mechanisms of the arsenic [especially As (Ⅲ)] removal. The floc samples were collected from two drinking water plants using IRB (Jyoyo and Yamatokoriyama, Japan), and our pilot - scale test site where arsenic and iron removal using IRB is under way (Mukoh, Japan). The Jyoyo and Yamatokoriyama IRB floc samples were subjected to As (Ⅲ) and As(Ⅴ) sorption experiments. The elemental composition of the floc samples was measured. XANES spectra were collected on As, Fe and Mn K-edges at synchrotron radiation facility Spring 8 (Hyogo, Japan). FT-IR and the X-ray diffraction spectra of the samples were also obtained. The IRB floc contained ca. 35 % Fe, 0.3%-3.5% Mn and 2%-6% P. The samples were highly amorphous and contained ferrihidrites and hydrated iron phosphate. According to XANES analyses of IRB, As associated with IRB was in +5 valence state when As (Ⅲ) (or As (Ⅴ)) was added in laboratory sorption test, Fe in +3 valence state, and Mn a mixture of+3 and +4 valence states. Small shift was observed in the XANES spectra of IRB on As K-edge as the equilibration time of the sorption experiment was increased. Gradual oxidation of a small amount of As (Ⅲ) associated with IRB or change in arsenic binding with sorption site were the probable mechanism. 相似文献
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56.
Jin-Soo Lee Kyung-Seok Ko Tong-Kwon Kim Jae Gon Kim Seong-Hyun Cho In-Suk Oh 《中国地球化学学报》2006,25(B08):152-152
The regional survey of groundwater used as a small water supply system was performed to know the effect of geology, soil properties and land use on groundwater quality at Nonsan City, Korea. A total of 126 groundwater samples were collected and analyzed at the study area. The multivariate statistical methods, principal components analysis and discriminant analysis, and GIS technique were used for the quantitative interpretation of groundwater quality. The study area is mainly composed of Precambrian gneiss, Jurassic granite, and Cretaceous volcanics, and metasedimentary rocks of the Ogcheon zone. The land use was grouped as paddy, upland, grassland, resident, point source, industrial area, and water system. The soil properties were classified as 4 major groups, Entisols, Alfisols, Inceptisols, and Ultisols, by the degree of development, and reclassified as 11 subgroups. The modified and simplified geologic map, soil map, and land use map were made by using ARCGIS soft-ware. The area of geology, soil property, and land use affecting the groundwater quality for each well were also calculated by ARCGIS soft-ware to acquire the quantitative parameters for multivariate statistical analysis. The monitoring results of groundwater in the study area showed that 13%-21% of the groundwater samples exceeded the portable water guideline and the main causes were turbidity, bacteria, arsenic and nitrate-N. The spatial distribution of each component showed the close relationship between groundwater quality and geology reflecting the topography, land use. 相似文献
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60.
Mihael Brencic 《Environmental Geology》2006,49(6):804-813
During the planning, designing, construction, operation and maintenance of highways, groundwater can be of important environmental
and constructional constraint that can significantly influence the safety operation of traffic and of big influence on the
operational costs of highways. To classify and conceptualize the relation between groundwater and highways, three important
groups of problems can be determined: groundwater protection from highway influences, protection of highway from groundwater
and economic use of groundwater for highway operation. In the present study, groundwater management strategies are represented
during all life cycles of highways. Greater emphasis is given to groundwater protection and field hydrogeological investigations
for proper groundwater management related to the highway. The approach adopted in Slovenia and the role of hydrogeology is
given as an illustration. 相似文献